I can't think of a way you could click ANYWHERE and trigger a sample as I don't think there's an action like that.
I know you can click on the little black square in ReaSamplOmatic to trigger the sample. I imagine most other Sampler VST's have a similar preview feature.
If you wanted to record what you're clicking you could set up the Virtual MIDI keyboard as your MIDI input for a track with ReaSamplOmatic on it, arm the track, press Record and click the keyboard to both trigger the sample and record the MIDI note.
Hope that helps some.
cheers,
argee
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