You can't use the double-sized icons with different pngs by default, you have to go to Color Themes folder in C:\Users\User\AppData\Roaming\REAPER\Data\toolbar_ icons and then look for the toolbar blank pngs, and create your own colorful icons from colored toolbar blank templates that can be found in most themes, there's also 2500 icons uploaded in the stash
But to change toolbar text colors, use the theme development tool, show theme and configuration window, and the text color can be changed in those options.
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